This disclosure sets forth a method for processing metal waste incorporating substantial zirconium as exemplified by nuclear fuel rods which include enriched uranium and other nuclear products. This process contemplates conversion of the zirconium and other constituents into oxides by mixing with an acid, subsequently forming a solution or a gel which is either dried or frozen, thereby yielding a green shaped body. The green body is thereafter sintered to form a dimensionally and structurally stable monolith for disposal.