In a process for producing a nitrile compound comprising introducing a
carbon ring or heterocyclic compound having organic substituents, ammonia
and the air into a reactor and reacting the introduced compounds in the
presence of a catalyst, during the reaction, a residual gas obtained
after the formed nitrile compound is separated from a reaction gas
discharged from the reactor is recycled to the reactor in an amount of 10
to 60% by volume based on the amount of the fresh raw material gas
supplied to the reactor and the ratio of the amount by mole of molecular
oxygen to the amount by mole of the organic substituent in the carbon
ring or heterocyclic compound having organic substituents supplied to the
reactor (O.sub.2/organic substituent) is kept within 1.5 to 7. The
reaction is achieved under an advantageous condition and the nitrile
compound can be produced industrially advantageously at a higher yield.