One embodiment of the present invention provides a process for fabricating an electrode for a capacitor using carbon nanotubes (CNTs), wherein the electrode comprises a metal substrate and a layer of active material (CNTs) coated onto the metal substrate. Specifically, the process starts by dispersing CNTs in a solvent to form a suspension. Next, the CNTs are charged in the suspension. The metal substrate is then immersed in the suspension. Next, the CNTs are deposited onto the metal substrate using electrophoretic deposition (EPD) to form the layer of active material on the metal substrate. In particular, the layer of active material is formed on the metal substrate without using a binder, which effectively reduces contact resistance between the active material and the metal substrate.