An interactive combination of Phoswich detector array (PDA) and differential absorption lidar (DIAL) is proposed to trace the unknown radioactive plumes released into the atmosphere from a reactor stack, containment of the nuclear power plants, radioisotope separation laboratories, reprocessing plants or the uranium conversion facilities. The hybrid system represents a powerful technique for the prompt identification and quantification of the effluents with various radionuclide contents to determine the corresponding external dose rate accordingly.