A method of preparing an actinide nitride fuel for nuclear reactors is
provided. The method comprises the steps of a) providing at least one
actinide oxide and optionally zirconium oxide; b) mixing the oxide with a
source of hydrogen fluoride for a period of time and at a temperature
sufficient to convert the oxide to a fluoride salt; c) heating the
fluoride salt to remove water; d) heating the fluoride salt in a nitrogen
atmosphere for a period of time and at a temperature sufficient to
convert the fluorides to nitrides; and e) heating the nitrides under
vacuum and/or inert atmosphere for a period of time sufficient to convert
the nitrides to mononitrides.