A serially connected organic electroluminescence device (SC-OELD) comprises the first OELD unit, the second OELD unit and a connecting layer disposed between the first OELD unit and second OELD unit. A method for improving color-shift of the SC-OELD, comprises: determining the color-shift tendencies of the first OELD unit and the second OELD unit, respectively, according to the different currents passing through the first OELD unit and second OELD unit; and combining the first OELD unit and the second OELD unit with the different color-shift tendencies, whereby the different color-shift tendencies of the first OELD unit and the second OELD unit are compensated each other while the electric charge is applied to the SC-OLED, so as to obtain a substantially pure color of the SC-OELD.