Disclosed is a one-pack type dental adhesive composition comprising: (a) 1.0 to 40.0 parts by weight of a silane coupling agent, (b) 0.01 to 0.4 part by weight of a weak acidic compound which is at least one of organic acid, boric acid and silicic acid, and has an acid dissociation exponent pKa of 3 or more in the form of an aqueous solution, (c) 0.01 to 0.4 part by weight of a strong acidic compound which is at least one of HF, HCl, HBr, HI, HNO.sub.3, HClO.sub.3, HClO.sub.4, HBrO.sub.4, HMnO.sub.4, H.sub.2SO.sub.4 and H.sub.3PO.sub.4 and has an acid dissociation exponent pKa of less than 3, (d) 0.1 to 5.0 part by weight of water, and (e) 20.0 to 99.0 parts by weight of a volatile organic solvent.