An ink composition is disclosed which contains at least one novel dye (CU)n(SAU)m that is capable of self-assembling under appropriate conditions to form supramolecular structures. More than one novel dye (CU)n(SAU)m and/or at least one non-colored self-assembling compound (SAU)p(X)q may be incorporated in these supramolecular structures. Also disclosed is an ink-jet printing process using these novel dyes, and an ink-jet printing apparatus provided with an ink cartridge containing such a dye.

 
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