A repeated "soak and dry" selectivation process for preparing a modified
metallosilicate catalyst composite is disclosed comprising of a mixture
of amorphous silica, alumina and a pore size controlled metallosilicate
useful for alkylaromatic conversion. The process comprises (a) contacting
an intermediate pore metallosilicate with an organosilicon compound in a
solvent for a specific duration and then recovering the solvent, (b)
combining the organosilicon compound treated metallosilicate with water
and then drying the catalyst, (c), repeating the steps a) and b) above
and (d) calcining the catalyst in an oxygen containing atmosphere
sufficient to remove the organic material and deposit siliceous matter on
the metallosilicate. In a another embodiment, when the organosilicon
compound is water soluble, step (b) may be avoided.